The actress said she was hampered by laryngitis when she auditioned for the part in Tom Hooper's critically-acclaimed production.
But having seen the film, Johansson conceded she could not have performed any better than Anne Hathaway, who won a Bafta for her role in the film.
"It was perfect and I think fateful and meant to be," she told Broadway.com.
"I auditioned with laryngitis. I did everything I could to, like, not have laryngitis. I sang my little heart out," she said.
"I think, looking at the film now, there's no possible way I ever could have topped that performance."
Johansson, currently starring in a Broadway production of Cat on a Hot Tin Roof, said the audition for Les Miserables "brought back so many memories" from when she tried out for the role of Cosette as a child.
"It was fun for me to revisit that," she added. "The jazz hands kid inside me was just over the moon!"
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